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The pure rotational and rotation‐vibrational Raman spectra of HCN and DCN have been photographed using a previously described instrument [7]. The molecular constants derived for HCN are in excellent agreement with those obtained from microwave and infrared spectroscopy. Especially, the measurements of the v 1 rotation‐vibrational Raman band have confirmed the hitherto indirectly obtained values for the molecular constants of the v1 vibrational state of HCN.
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Bendtsen et al. (1974) studied this question.
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