The method of Stogryn and Hirschfelder, which divides two-particle phase space into bound, metastable, and free particle parts, is applied to the statistical averages which determine the first three spectroscopic moments of ``collision-induced'' far-infrared and Raman spectra. Numerical results are presented for a number of models of noble gas systems. It is shown that for some systems, but not all, dimers make important, although not necessarily well-separated, contributions to the spectrum.
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Howard B. Levine (1972) studied this question.
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