Temperature matters! The separation efficiency of complex mixtures of gases (acetylene, carbon dioxide, methane, nitrogen) and vapors (benzene, cyclohexane) by adsorption on A[Cu3(μ3-OH)(μ3-4-carboxypyrazolato)3] (A@1) metal–organic frameworks depends on temperature and the extraframework cation A (see picture). NH4@1 also behaves as an oxidation catalyst.
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Procopio et al. (2010) studied this question.
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