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August 22, 2026OpticaOpen Access

Nanoscopy of surface polarization with oblique dipole orientations

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Authors

VDV. G. M. DuarteDMD. A. MirandaDCD. F. P. Cunha

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Overview

Theoretical modeling reveals that near-field nanoscopy resolves oblique dipole orientations in 2D materials, indicating enhanced sensitivity compared to conventional far-field reflectance.

Key Points

  • To establish electrodynamic boundary conditions for confined dipoles with arbitrary orientations on planar and cylindrical surfaces and assess their detection using near-field optical techniques.
  • Derived analytical boundary conditions and loss functions for surface dipole sheets with arbitrary in-plane and out-of-plane orientations.
  • Modeled optical reflectance and scattering-type scanning near-field optical microscopy (s-SNOM) point-dipole responses, validating against experimental data for monolayer tungsten diselenide (WSe2).
  • Large dipole strengths split the dipole oscillation reflectance peak and generate pairs of polaritonic resonances in the loss function from coupled in-plane and out-of-plane components.
  • The s-SNOM point-dipole model exhibited dual distinct peaks sensitive to dipole obliqueness, with an oblique dipole angle of 5.7° significantly improving fit to experimental monolayer WSe2 data.

Cite This Study

Duarte et al. (2026) studied this question.

synapsesocial.com/papers/6a895e6bca7ade938187c90ehttps://doi.org/10.1364/optica.599585
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