We have studied the subpicosecond gain dynamics of XeCl and KrF with the following results for XeCl (KrF): saturation energy density 0.85 (2.0) mJ/cm2, small-signal-gain coefficient 0.12–0.15 (0.20–0.22) cm−1, gain recovery of 62% (25%) with a time constant of 52 (54) psec. A molecular reorientation time of ≈1 psec was observed in both excimers.
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Szatmári et al. (1987) studied this question.
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