The density matrix formalism describing the interaction between a three level molecular system and two nearly resonant laser fields of arbitrary intensity is extended to include the molecularM-level degeneracy. Expressions for gain on the two possible relative polarizations of a laser pumped molecular laser are derived and its saturation behavior discussed. Numerical results for the 385 μm transition in D2O and 496 μm transition in CH3F are presented.
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Drozdowicz et al. (1979) studied this question.
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