Infrared laser beams at 3.095 μ in helium-buffered cesium vapor and at 2.254 and 2.293 μ in helium-buffered rubidium vapor have been produced by irradiating these gases with beams from various giant pulse lasers. The mechanism of excitation is shown to involve two-step photodissociation of Cs2 and Rb2 molecules.
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Sorokin et al. (1969) studied this question.
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