Spectroscopic analysis identifies intermolecular vibration bands in pyridine halogen complexes, indicating a three-centre molecular orbital treatment explains their bonding behavior.
The intermolecular vibration band has been identified in the far infra-red spectra of the pyridine IBr and pyridine ICI charge transfer complexes. All the reported observations on these and similar complexes can be accounted by a simple 3-centre molecular orbital treatment.
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Ginn et al. (1966) studied this question.
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