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Single crystals of Pb (NO3)2 and Sr (NO3)2 X‐irradiated at 90 °K are studied using electron spin resonance. The spectra of paramagnetic species having hyperfine structure due to a single nitrogen nucleus are measured at 90 °K. The principal values of g‐tensors and hyperfine tensors are determined; also the directions of their principal axes. The species in both crystals are tentatively assigned to NO2‐3. In the crystals of Pb(NO3)2, the superhyperfine structure assigned to the interaction with three Pb nuclei is also studied, and the principal tensor values of this superhyperfine interaction and the directions of their principal axes determined.
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Žďénský et al. (1964) studied this question.
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