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The polymerization rate of two binary monomer systems styrene (St)/N‐vinyl‐2‐pyrrolidone (NVP) and NVP/methyl methacrylate (MMA) was investigated dilatometrically in bulk at 60°C with AIBN as initiator. While the copolymerization rate of the system St/NVP can be satisfactorily described by means of the classical reaction model, this is not the case for the system NVP/MMA. This deviation from the classical model can be explained by a charge‐transfer interaction between NVP and MMA which was measured by means of 1H and 13C NMR spectroscopy.
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Braun et al. (1987) studied this question.
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