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Formulations are examined for connecting average kinetic energies of the products of a unimolecular decomposition with the total available energy. A straightforward method for the calculation of kinetic shifts is then described. Existing data suggest, nevertheless, that the effective number of internal degrees-of-freedom for energy disposal may be greater than the physical number, a result inaccessible to existing theory. A formal reconciliation is indicated here.
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Cornelius E. Klots (1973) studied this question.
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