Optical third-harmonic coefficients are calculated for the inert gases and are compared with recent experimental values. We find them to range from 0.9×{}10^-39 esu/atom for He to 222×{}10^-39 esu/atom for Xe. Our calculated values, expressed as ratios to the optical third-harmonic coefficient of He, compare favorably with one of two sets of recently reported experimental values.
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E. Dawes (1968) studied this question.
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