Competition between three-photon resonantly enhanced vacuum ultraviolet third-harmonic generation and six-photon multiphoton ionization using the A state in gaseous carbon monoxide is observed. Excitation spectra of the third-harmonic emission exhibit increasing blue shifts and broadening with increasing pressure due to the phase matching requirements. Estimates for the efficiency and tunability show that third-harmonic generation in carbon monoxide molecules is a promising source for coherent vacuum ultraviolet light.
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Glownia et al. (1982) studied this question.
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