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A method of inferring the principal values and the directions of the principal axes of the g -tensor for a paramagnetic complex in a single crystal from measurements of the g -value variation in three different planes is described, and an ambiguity in the determination of the principal values that will often arise in practice is pointed out and discussed. An estimate of the root mean square error in the determination is given.
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D. S. Schonland (1959) studied this question.
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