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Polymerization processes of high polymers are investigated using matrix method of the Ising model. It is shown that information on the polymerization mechanisms can be obtained from the data of high resolution nuclear magnetic resonance spectroscopy. Polymerization of two component co-polymers and asymmetric polymerization are examined. The reality of penultimate effect is also discussed. Physical quantities such as monomer reactivity ratios and persistence ratios of asymmetrically polymerized samples are given explicitly as functions of the intensity of nuclear magnetic resonance spectra and also, in some cases, of polymerization temperature.
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Riichirǒ Chûjô (1966) studied this question.
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