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An electrochemical meta -C–H silylation of pyridines with readily available hydrosilanes is described. The reaction proceeds under mild conditions without noble metal catalysts or external oxidants using N -hydroxyphthalimide as a hydrogen-atom-transfer catalyst. In addition, quinolines and pyrazines are well tolerated, affording the corresponding silyl-functionalized azines.
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Yang et al. (2025) studied this question.
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