► Multiple-hole oxidation process is the bottleneck for solar fuel synthesis. ► Formation of higher carbon chain is usually very difficult caused by weakly bonded CO. ► A new strategy couples the photoreduction of CO 2 with water photolysis. ► Junction photocatalyst system performs much better than single materials. ► Solid-state mediator is proven effective as alternative liquid mediators.
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Handoko et al. (2013) studied this question.
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