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January 1, 2017Polymer Chemistry

Ab initio based kinetic Monte Carlo analysis to unravel the propagation kinetics in vinyl acetate pulsed laser polymerization

Gilles Desmet Yoshi W. Marien Paul Van Steenberge Dagmar D’hooge Marie‐Françoise Reyniers Guy Marin

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Abstract

The radical propagation kinetics of vinyl acetate in pulsed laser polymerization (PLP) is studied by combining ab initio calculated rate coefficients with kinetic Monte Carlo modeling of PLP spectra.

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Desmet et al. (2017) studied this question.

synapsesocial.com/papers/6a962cfa72ac8e1ccf902d32 https://doi.org/10.1039/c7py01008g

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Synapse has enriched 5 closely related papers on similar clinical questions. Consider them for comparative context:

1The laser‐flash‐initiated polymerization as a tool of evaluating (individual) kinetic constants of free‐radical polymerization, 2. The direct determination of the rate of constant of chain propagationOriginal Research · 1987 · 404 citations
2Kinetics of laser-initiated polymerization and molecular-weight distribution of the resultant polymerOriginal Research · 1977 · 47 citations
3Determining Free‐Radical Propagation Rate Coefficients with High‐Frequency Lasers: Current Status and Future PerspectivesOriginal Research · 2015 · 31 citations
4Copolymerization Kinetics of Methyl Methacrylate−Styrene Obtained by PLP-MALDI-ToF-MSOriginal Research · 2006 · 49 citations
5Effect of Head-To-Head Addition on Vinyl Acetate Propagation Kinetics in Radical PolymerizationOriginal Research · 2014 · 24 citations

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