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Energy storage and disposal by electron transfer in molecular and supermolecular systems may provide a conceptual and technical basis for the construction of molecular electronic devices, e.g., molecular wires and switches. We consider structural, intramolecular, medium energetic and medium dynamic control of electron transfer in synthetic and neutral supermolecules. Optimization principles are formulated for ultrafast, highly efficient and stable charge separation.
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Jortner et al. (1993) studied this question.
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