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February 16, 2007Angewandte Chemie

A Concise, Biomimetic Total Synthesis of Stephacidin A and Notoamide B

Thomas J. Greshock Alan W. Grubbs Sachiko Tsukamoto Robert M. Williams

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Abstract

Die Natur kopiert: Eine biomimetische Totalsynthese von Stephacidin A gelang mithilfe einer intramolekularen Diels-Alder-Reaktion. Anschließend wurde Stephacidin A in einem Schritt durch Oxaziridin-vermittelte Oxidation in Notoamid B überführt, womit erstmals die biomimetische Totalsynthese von Notoamid B gelungen ist (siehe Schema).

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Greshock et al. (2007) studied this question.

synapsesocial.com/papers/6a973f81362b708b0889a9ca https://doi.org/10.1002/ange.200604378

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