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Ar and CO 2 physisorption on a very well crystallized sample of fullerene C 60 was studied by means of Monte Carlo computer simulations. Ar and CO 2 experimental isotherms were determined on high-purity C 60 to fit the potential parameters. Analysis of the structure of the adsorbed film indicated that both gases are adsorbed in the voids of the C 60 structure in a solid state with densities slightly larger than the bulk solid. Both gases exhibited a behavior similar to nitrogen. The cross-sectional area found for Ar is 0.121 nm 2 . The existence of three adsorption sites found previously has been confirmed.
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Martı́nez-Alonso et al. (2000) studied this question.
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