Supramolecular solids are an ideal medium for time-resolved diffraction studies at atomic resolution as they allow dilution of the active species, and the study of a species in different states of aggregation and different environments, but attention must be paid to excited-state quenching due to energy transfer. Crystallinity must be preserved up to reasonable product concentrations if chemical reactions are to be monitored at the atomic level.
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Coppens et al. (2006) studied this question.
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