We report a one-step method of assembling supramolecular colloidosomes at the interface of microfluidic droplets. The self-assembly process utilises a versatile CB[8] host-guest system to reversibly crosslink polystyrene nanoparticles via a polyacrylamide linker. These micrometre-sized hollow structures can be loaded with water-soluble cargo during formation, which can then undergo triggered release.
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Stephenson et al. (2014) studied this question.
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