A high-resolution study of the rotational Raman spectra of cyclopropane and cyclopropane-d6 has yielded the values 0.66962 ± 0.00020 cm−1 and 0.46079 ± 0.00015 cm−1 for their ground-state rotational constants. From these values the C–C internuclear distance is determined to be 1.514 ± 0.002 Å.
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Jones et al. (1964) studied this question.
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