We present picosecond time-resolved pump-probe measurements of the photodissociation and recombination dynamics of I−2 surrounded by a specific number of CO2 molecules in mass selected I−2 (CO2)n clusters. The transient bleaching data can be fit to an exponential absorption recovery of 30±10 ps in I−2 (CO2)9 clusters and 10±5 ps in I−2 (CO2)16 clusters. The data demonstrate the feasibility of measurements of real-time reaction dynamics in microsolvent environments.
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Ray et al. (1989) studied this question.
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