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An improved version of an earlier Larson-type model of solution of amphiphiles is used to simulate the spontaneous formation of vesicles. Starting with a solution of amphiphiles either uniformly distributed or aggregated in an ordered way, self-organization into vesicles was observed by carrying out extensive Monte Carlo simulations. The aggregation of single-tailed amphiphiles and the role of the bending rigidity in the chains are also discussed.
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Américo Tristão Bernardes (1996) studied this question.
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