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A simple spectrophotometric method for the evaluation of formation constants for aqueous copper(I) has been developed, based on the kinetics of reduction of Co(III)(NH(3))(5)X complexes. The method has been applied to the aqueous copper(I)-acetonitrile system to determine the successive formation constants beta(1), beta(2), and beta(3) as 4.3 x 10(2) M(-)(1), 1.0 x 10(4) M(-)(2), and 2.0 x 10(4) M(-)(3), respectively, in 0.14 M NaClO(4)/HClO(4) at 21 +/- 1 degrees C.
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Kamau et al. (2001) studied this question.
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