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We have studied the dynamics of two-electron wave packets in barium consisting of 6snd1,3D₂ Rydberg states, which are degenerate with the doubly excited 5d7d¹D₂ state. The configuration interaction manifests itself in the temporal oscillation of the wave packet among the three configurations in this system. We present in detail a quantum defect theory analysis that adequately describes the system, and we introduce a simple physical picture to understand the dynamics.
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Lyons et al. (1998) studied this question.
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