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Well-defined statistical copolymers of vinyl acetate and 1-(trifluoromethyl)vinyl acetate were synthesized by RAFT/MADIX polymerization. These copolymers exhibited enhanced solubilities in supercritical CO 2 compared to poly(vinyl acetate). A copolymer composition–solubility optimum was observed, which resulted from a subtle interplay between polymer–polymer interactions and entropy of mixing.
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Girard et al. (2012) studied this question.
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