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New bis(β-diketonato)Cr(III) and Ni(II) complexes with a chelating nitronyl nitroxide radical were synthesized and characterized. The intensification and/or large Stokes shift of the spin-forbidden components and the charge transfer transitions revealed by the resonance Raman spectra in the visible region were found, which result from the moderate exchange coupling.
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Yoshida et al. (1997) studied this question.
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