We report a new variant of the femtosecond transition-state spectroscopy technique−transient stimulated emission pumping (TSEP). The initial application of TSEP to studies of ozone visible photodissociation indicates that the molecule is trapped in the Franck–Condon region for ∼90 fs. The wave packet then spreads along the reaction coordinate.
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Chen et al. (1992) studied this question.
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