Impulsive stimulated resonance Raman scattering performed with femtosecond pulses comprises an all time domain Raman technique providing vibrational spectra of the ground state chromophore. We report the first application of this technique to record Raman free induction decays of nascent diiodide ions, undergoing rapid vibrational relaxation following triiodide photodissociation in ethanol solution.
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Banin et al. (1993) studied this question.
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