This communication describes the design of bifunctional VO(x)/TS-1 catalysts with enhanced redox and acidic character via doping SO(4)(2-) and PO(4)(3-) for selective oxidation of methanol to dimethoxymethane. Redox sites enable the production of formaldehyde, while acidic sites favor the condensation of formaldehyde to DMM.
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Chen et al. (2011) studied this question.
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