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conditions. Our results reveal that mobile ions accumulate at the PCs, triggering a faster degradation of the device. These observations are further supported by one- and two-dimensional drift-diffusion simulations that confirm the accumulation of ions at the PCs. This work, therefore, highlights the importance of ion management for improved stability and points to a new degradation mechanism when a discontinuous insulating layer forms at the perovskite interfaces.
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He et al. (2025) studied this question.
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