Spectroscopy study demonstrates preserved oxidation state sensitivity in stimulated manganese X-ray emission, indicating new avenues for high-resolution electronic structure analysis.
XES. The work builds on our previous observation that S-XES from Mn(II) and Mn(VII) complexes pumped at high intensities can exhibit stimulated emission without sacrificing the chemical sensitivity to oxidation states. This technique opens the door to controlled high-resolution electronic structure spectroscopy in transition-metal complexes beyond the core-hole lifetime, with potential applications in catalysis, inorganic chemistry, and materials science.
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Kröll et al. (2026) studied this question.
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