An explanation of a succesful empirical criterion for the phase of clusters produced in a supersonic jet is reexamined in the light of a kinetic prefactor for freezing proposed by Grant and Gunton. It is found that the Grant-Gunton theory accounts significantly more faithfully for the empirical criterion than does the theory of molecular jumps based on a model of viscous flow and confirms the essential correctness of the kinetic explanation.
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Lawrence S. Bartell (1996) studied this question.
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