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The authors report here the most comprehensive study to date of the coupling between magnetism and the crystal lattice in CoPS₃, a magnetic van der Waals material with high spin-orbit coupling and unquenched orbital moments. Employing a suite of experimental techniques, they uncover unambiguous signatures of spin-lattice coupling: magnetostriction and magnon-phonon hybridization. These findings illuminate the intricate interplay between the spin, orbital, and lattice degrees of freedom in this quasi-two-dimensional system.
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