Clusters in intense XUV pulses: Effects of cluster size on expansion dynamics and ionization

This is the authors' abstract. We don't add key points for this paper.

We examine the effect of cluster size on the interaction of Ar₅₅-Ar₂₀₅₇ with intense extreme ultraviolet (XUV) pulses, using a model we developed earlier that includes ionization via collisional excitation as an intermediate step. We find that the dynamics of these irradiated clusters is dominated by collisions. Larger clusters are more highly collisional, produce higher charge states, and do so more rapidly than smaller clusters. Higher charge states produced via collisions are found to reduce the overall photon absorption, since charge states of Ar²⁺ and higher are no longer photoaccessible. We call this mechanism collisionally reduced photoabsorption, and it decreases the effective cluster photoabsorption cross section by more than 30% for Ar₅₅ and 45% for Ar₂₀₅₇. The time evolution of the electron kinetic energy distribution begins as a (mostly) Maxwellian distribution. Further, the electron velocity distribution of large clusters quickly become isotropic while smaller clusters retain the inherent anisotropy created by photoionization. Last, the total electron kinetic-energy distribution is integrated over the spatial profile of the laser and the log-normal distribution of cluster size for comparison with a recent experiment [C. Bostedt et al., Phys. Rev. Lett. 100, 133401 (2008)], and good agreement is found.