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March 20, 2008Angewandte Chemie

Mass Spectrometric Screening of Chiral Catalysts by Monitoring the Back Reaction of Quasienantiomeric Products: Palladium‐Catalyzed Allylic Substitution

Constanze A. Müller Andreas Pfaltz

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Abstract

Fortschritt im Rückwärtsgang: Auf dem Prinzip der mikroskopischen Reversibilität beruht ein neues Screening-Verfahren für chirale Katalysatoren: Die intrinsische Enantioselektivität von Palladiumkatalysatoren in allylischen Substitutionen zeigt sich beim ESI-massenspektrometrischen Verfolgen der Rückreaktion ausgehend von quasienantiomeren Allylierungsprodukten (siehe Schema).

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Müller et al. (2008) studied this question.

synapsesocial.com/papers/6aa6dd060ab0fd924bf4d920 https://doi.org/10.1002/ange.200705081

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