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Abstract 1,2,2‐Trisubstituted aziridines have been prepared by reduction of secondary N‐1‐(2‐chloroalkylidene)amines with lithium aluminium hydride. N‐Substituted 1‐azaspiro[2.5]octanes (spiroaziridines) have been synthesized by this method. Under appropriate gas chromatographic conditions, 1,2,2‐trisubstituted aziridines underwent rearrangement to the corresponding secondary N‐1‐(alkylidene)amines. The reaction mechanisms are discussed.
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Kimpe et al. (1977) studied this question.
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