The paper presents results of a high-pressure, non-self-sustained crossed discharge– M = 3 supersonic laser cavity operation. A stable and diffuse pulser–sustainer discharge in O 2 –He flows is generated at pressures of up to P 0 = 120 Torr and discharge powers of up to 2.1 kW. The reduced electric field in the dc sustainer discharge ranges from 0.6 × 10 −16 to 1.2 × 10 −16 V cm 2 . Singlet delta oxygen (SDO) yield in the discharge, up to 5.0–5.7% at the flow temperatures of 400-420 K, was inferred from the integrated intensity of the (0, 0) band of the O 2 ( a 1 Δ → X 3 Σ) infrared emission spectra calibrated using a blackbody source. The yield increases with the discharge power and remains nearly independent of the O 2 fraction in the mixture (in the 10–20% range). Static pressure and temperature measurements in the supersonic cavity show that a steady-state M = 3 flow in the cavity can be sustained for up to 20 s, at the flow temperature of T = 120 ± 15 K. The results suggest that the measured SDO yield exceeds the threshold yield at the cavity temperature by up to a factor of 2.5. PLIF iodine vapour visualization in the supersonic cavity, which showed the presence of large-scale structures, suggests the need to improve iodine vapour mixing with the main oxygen–helium flow.
No takes yet. Share an insight, caveat, or question.
Hicks et al. (2007) studied this question.
Synapse has enriched 5 related papers. Consider them for comparative context: