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A study of the mechanisms of spin delocalization to γ hydrogens was conducted by investigating the change in spin density distribution upon geometrical deformation. The mechanisms are expressed in valence bond pictures. The spin densities were calculated using the SCF-MO-INDO method for the propyl radical. An empirical expression for γ-hydrogen hfsc's is proposed.
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Underwood et al. (1973) studied this question.
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