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Nitrobenzene ions, energy selected by photoelectron–photoion coincidence (PEPICO), are photodissociated by a pulsed dye laser. The time-delayed laser pulse is triggered by the detection of a zero energy electron indicating the formation of an ion of known internal energy. A detailed description of the experimental requirements is presented. This first report of the combination of PEPICO with ion photodissociation includes the determination of the nitrobenzene ion photodissociation cross section of (6±2)×10−19 cm2, and the study of kinetic energy released in that dissociation. Applications for other uses are discussed.
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Bunn et al. (1986) studied this question.
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