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This review summarizes theoretical formulations of resonance Raman scattering that express the steady-state spectrum in terms of time-dependent quantities. Time-domain expressions for the Raman or direct one-photon absorption (electronic or vibrational) lineshape are compared and contrasted with time-dependent formulations for the resonance Raman intensity. Time-domain expressions that properly describe the total spontaneous emission of a chromophore interacting with a bath are also discussed. A final section addresses a few aspects of the interpretation and practical application of these theories to real experimental data.
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Anne B. Myers (1997) studied this question.
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