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The rate constant for vibrational-vibrational exchange, K 10 01 = (1 ± 0.4) × 10 −13 cm 3 /sec, was determined under conditions of selective biharmonic excitation of the first vibrational state of nitrogen. Procedural aspects of measurements of the vibrational relaxation time under biharmonic excitation conditions are discussed.
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Valyanskiĭ et al. (1984) studied this question.
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