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September 5, 2025InfoMatOpen Access

Reallocation of active lithium by regulating electrochemical structural connectivity in anode‐free lithium metal batteries

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Authors

JZJinqi ZhuNortheast Forestry UniversityWGWenxin GouDonghua UniversitySHS. Y. HuangPanzhihua University

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Overview

This research demonstrates the correlation between electrochemical structural connectivity and active Li loss pathways in anode-free lithium metal batteries, indicating improved performance.

Key Points

  • The regulated Li growth process results in minimized irreversible Li loss at only 0.003 mg per cycle.
  • Anode-free LiFePO4 pouch cells show a retention of 61.4% initial reversible capacity after 100 cycles.
  • Insights from optimizing Li nucleation lead to improved active Li utilization in anode-free lithium metal batteries.
  • High-density spatial multidimensional nucleation enhances electronic pathways and interfacial mass transfer.

Cite This Study

Zhu et al. (2025) studied this question.

synapsesocial.com/papers/68bb3a432b87ece8dc9555f7https://doi.org/10.1002/inf2.70067
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