Analysis demonstrates 95.19% selectivity for ethylene in 1,2-dichloroethane transformation over Co-N4 sites, suggesting influence of peripheral structures.
The role of remote nonmetallic species remains underexplored for 1,2-dichloroethane (DCE) electrochemical dechlorination over single-metal sites. We demonstrated that a peripheral conjugated structure and nitrogen atoms accelerate the transformation of *CH2CH2Cl to *CH2CH2 and ethylene desorption. CoPc achieved an FEethylene of 95.19 ± 0.02% and a 75.8-fold increase in Jethylene.
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Long et al. (2025) studied this question.
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