This work demonstrates chlorine-mediated electrocatalytic methane valorization, indicating a novel site engineering strategy.
Cl desorption energy (0.27 eV) to suppress over-dehydrogenation. This work establishes a *Cl-mediated dual-site pathway for electrocatalytic methane valorization, offering a promising strategy for mediator-guided active site engineering in challenging inert-alkane valorization.
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Qian et al. (2026) studied this question.
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