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Asymmetric synthesis achieved tricyclic skeleton of erectcyanthin C, highlighting its role in anti-dyslipidemic activity.
The stereoselective asymmetric synthesis of the tricyclic skeleton of erectcyanthin C, a cyathane diterpenoid exhibiting anti-dyslipidemic activity, is reported. The synthetic strategy features the regioselective formation of vinyl triflate through Sakurai allylation/reductive debromination followed by gold-catalyzed stereoselective Nazarov cyclization and late-stage ring-closing metathesis.
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Sang et al. (2025) studied this question.
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