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This is a Quantitative Study study.

Accelerating Electrochemical Hydrogen Evolution by Introducing Local Proton Source in Non‐Heme Iron (III) Complexes

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This research demonstrates improved catalytic activity for hydrogen evolution in Fe III complexes, indicating the role of ligand modifications.

Complex 1 exhibits superior electrocatalytic activity for hydrogen evolution reaction with a k cat of 1.4 ± 0.07 × 10 5 M −1 s −1.
Internal hydroxy groups in complex 1 facilitate intramolecular proton transfer, enhancing catalytic rates for hydrogen evolution.
Synthesis involved characterizing three non-heme Fe III complexes through various spectroscopic methods to analyze their properties.
Modifying ligand scaffolds in Fe III complexes may lead to significant changes in their hydrogen evolution catalytic activity.

Bharath et al. (2025) studied this question.

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This research demonstrates improved catalytic activity for hydrogen evolution in Fe III complexes, indicating the role of ligand modifications.